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Glassy Nuclei in Amorphous Ice

Glassy Nuclei in Amorphous Ice

Christina Maria Tonauer

67,98 €
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Editorial:
Springer Nature B.V.
Año de edición:
2019
Materia
Química física
ISBN:
9783658263232
67,98 €
IVA incluido
Disponible

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Sobre IBD

Christina Maria Tonauer finds novel evidence for the first-order nature of the transition between high-density amorphous ice (HDA) and low-density amorphous ice (LDA), supporting water’s liquid-liquid transition scenarios. Pressure-dependent crystallisation experiments of differently prepared expanded high-density amorphous ice samples (eHDA) and subsequent powder x-ray diffraction experiments disclose nucleation of LDA domains in bulk HDA, a typical feature of a first-order transition. The comparison of pressure-dependent crystallisation temperatures of eHDA samples with LDA nuclei and bulk LDA allows the estimation of the Laplace pressure and the size of a LDA nucleus.

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